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Cu(I) catalyst, sulfonyl azide and alkyne generate ketenimine intermediate after releasing N2 gas. This electrophilic ketenimine intermediate reacts with amines and to generate asymmetric imines as products. Chang's group also showed water, alcohols, the C3 position of pyrrole and other nucleophiles can be used in this reaction.
325:
Cu-catalyzed multicomponent coupling is a notable process developed by Chang's group. In 2005, they published a highly efficient and mild catalytic three component coupling between an alkyne, sulfonyl azide, and amine. Unlike click chemistry which generates 1,4-triazoles as products, in this case a
293:
as an assistant professor, and moved to KAIST as a full professor in 2002. In 2012, he was selected as a director of the Center for
Catalytic Hydrocarbon Functionalizations at the Institute for Basic Science, which is the biggest Korean government funded research institute. He also has been working
352:
In 2016, Chang's group discovered new nitrogen sources. Their new nitrene precursor, 1,4,2-dioxazol-5-one, is more convenient to prepare, store and use compared to azides. Moreover, it has a strong affinity to the rhodium or
Iridium metal center, and thus gives excellent amidation efficiency. They
341:
Rhodium or iridium catalyzed C-H amidation and amination are other achievements of his group. In 2012, his group published rhodium catalyzed intermolecular amidation of arenes using sulfonyl azide as a nitrene precursor. This reaction generates N2 as the single byproduct, doesn't need external
309:
Chang's group studies new organic reactions and mechanisms with transition metal catalysis. In particular, his group contributed to the development of "copper catalyzed multicomponent coupling" in the 2000s. Since 2008, his group has focused on C-H functionalization and made a number of
785:
Yoo, Eun Jeong; Ahlquist, Mårten; Bae, Imhyuck; Sharpless, K. Barry; Fokin, Valery V.; Chang, Sukbok (July 2008). "Mechanistic
Studies on the Cu-Catalyzed Three-Component Reactions of Sulfonyl Azides, 1-Alkynes and Amines, Alcohols, or Water: Dichotomy via a Common Pathway".
342:
oxidant, has broad substrate scope and high functional group tolerance. Chang's group advanced their work by using different directing groups, different azides and various substrates. They also published that iridium also works well for C-H amidation/amination.
872:
Kim, Ji Young; Park, Sae Hume; Ryu, Jaeyune; Cho, Seung Hwan; Kim, Seok Hwan; Chang, Sukbok (2012-05-24). "Rhodium-Catalyzed
Intermolecular Amidation of Arenes with Sulfonyl Azides via Chelation-Assisted C–H Bond Activation".
1178:
Park, Yoonsu; Park, Kyung Tae; Kim, Jeung Gon; Chang, Sukbok (2015-03-30). "Mechanistic
Studies on the Rh(III)-Mediated Amido Transfer Process Leading to Robust C–H Amination with a New Type of Amidating Reagent".
653:
300:
since 2015. In 2023, he was selected to co-run the KAIST Cross
Generation Creation Lab, a laboratory designed to continue the know-how of professors about to retire through collaboration with younger professors.
1222:
Park, Yoonsu; Heo, Joon; Baik, Mu-Hyun; Chang, Sukbok (2016-10-13). "Why is the Ir(III)-Mediated Amido
Transfer Much Faster Than the Rh(III)-Mediated Reaction? A Combined Experimental and Computational Study".
1134:
Kang, Taek; Kim, Youngchan; Lee, Donggun; Wang, Zhen; Chang, Sukbok (2014-03-05). "Iridium-Catalyzed
Intermolecular Amidation of sp3 C–H Bonds: Late-Stage Functionalization of an Unactivated Methyl Group".
1502:
699:
Bae, Imhyuck; Han, Hoon; Chang, Sukbok (February 2005). "Highly
Efficient One-Pot Synthesis ofN-Sulfonylamidines by Cu-Catalyzed Three-Component Coupling of Sulfonyl Azide, Alkyne, and Amine".
1610:
391:
742:
Cho, Seung Hwan; Yoo, Eun Jeong; Bae, Imhyuck; Chang, Sukbok (November 2005). "Copper-Catalyzed
Hydrative Amide Synthesis with Terminal Alkyne, Sulfonyl Azide, and Water".
829:
Cho, Seung Hwan; Chang, Sukbok (2008-03-31). "Room Temperature Copper-Catalyzed 2-Functionalization of Pyrrole Rings by a Three-Component Coupling Reaction".
1091:
Kim, Jinwoo; Chang, Sukbok (2014-01-27). "Iridium-Catalyzed Direct CH Amidation with Weakly Coordinating Carbonyl Directing Groups under Mild Conditions".
1045:
1713:
1678:
1323:
Park, Yoonsu; Chang, Sukbok (2019-02-18). "Asymmetric formation of γ-lactams via C–H amidation enabled by chiral hydrogen-bond-donor catalysts".
385:
81:
654:"Palladium-Catalyzed C−H Functionalization of PyridineN-Oxides: Highly Selective Alkenylation and Direct Arylation with Unactivated Arenes"
441:
403:
961:
Shin, Kwangmin; Baek, Yunjung; Chang, Sukbok (2013-06-20). "Direct CH Amination of Arenes with Alkyl Azides under Rhodium Catalysis".
498:
447:
243:
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1708:
356:
37:
221:; born August 1, 1962) is a South Korean organic chemist. He is a distinguished professor in the Department of Chemistry at
1703:
1611:"Seven IBS Scientists Named World's Most Highly Cited Researchers: Accounting for 13.1% of Korea's scientists on the list"
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Hong, Seung Youn; Park, Yoonsu; Hwang, Yeongyu; Kim, Yeong Bum; Baik, Mu-Hyun; Chang, Sukbok (2018-03-01).
1583:"IBS Places First Among Korean Institutions by Featuring 9 Scientists in List of Highly Cited Researchers"
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later published selective formation of gamma-lactams via C-H amidation with this type of nucleophile.
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2006: One of 50 Representative Research Performances, Korea Science & Engineering Foundation
229:(IBS) Center for Catalytic Hydrocarbon Functionalizations (CCHF). He was an associate editor on
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1005:"Rhodium-Catalyzed Direct Amination of Arene C-H Bonds Using Azides as the Nitrogen Source"
1268:"Selective formation of γ-lactams via C–H amidation enabled by tailored iridium catalysts"
8:
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453:
435:
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1503:"American and Korean Chemical Societies collaborate to recognize advancement of science"
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as a postdoctoral fellow from 1996 to 1998. In early 1998, he joined the faculty of
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1046:"Iridium-Catalyzed Direct Arene C–H Bond Amidation with Sulfonyl- and Aryl Azides"
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2003: Thieme Journals Award, Synlett/Synthesis Professorship Award in Asian Area
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1192:
1477:"Professor Chang, Sukbok received the ACS-KCS Excellence Award for 2017"
1366:
1423:"2019 Korea Best Scientist and Technologist Award, President of Korea"
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1061:
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2002: Young Chemist Award, Korean Chemical Society sponsored by WILEY
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for the carbon-carbon bond and carbon-heteroatom bond formation.
329:
1636:
1399:
431:
2016: Yoshida Prize, International Organic Chemistry Foundation
399:
2018: Korea Toray Science Award, Korea Toray Science Foundation
135:
652:
Cho, Seung Hwan; Hwang, Seung Jun; Chang, Sukbok (July 2008).
638:
1453:
1427:
IBS KAIST Center for Catalytic Hydrocarbon Functionalizations
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222:
151:
111:
67:
253:. His major research interest is transition metal catalyzed
313:
1044:
Lee, Donggun; Kim, Youngchan; Chang, Sukbok (2013-10-10).
388:, Korean Federation of Science and Technology Societies (
194:
784:
916:"Graphical Abstract: Angew. Chem. Int. Ed. 39/2012".
474:
2005: Shim Sang Cheol Award, Korean Chemical Society
235:and has served on the editorial advisory boards of
223:Korea Advanced Institute of Science and Technology
465:2010: KCS Academic Award, Korean Chemical Society
434:2015-2020: Highly Cited Researcher in chemistry,
1660:
1265:
1221:
1177:
613:"카이스트 김정호·장석복 교수팀, 학문의 대를 잇는 '초세대 협업연구실' 추가 개소"
462:, Kyung-Ahm Education & Cultural Foundation
1133:
741:
960:
871:
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468:2008: Star Faculty, Korea Research Foundation
386:Top Scientist and Technologist Award of Korea
330:Rhodium, Iridium-catalyzed C-N bond formation
84:(2019), Highly Cited Researcher (2015-2019),
82:Top Scientist and Technologist Award of Korea
529:"Sukbok Chang Wins Top Korean Science Prize"
522:
520:
442:Ministry of Science, ICT and Future Planning
389:
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216:
157:
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408:2018: Grand Academic Research Award, KAIST
404:Japan Society for the Promotion of Science
265:Sukbok Chang received his B.S degree from
36:
1322:
1291:
1020:
937:
517:
277:'s group and received his PhD in 1996 at
1714:Recipients of the Ho-Am Prize in Science
1679:Academic staff of Ewha Womans University
1641:Korean Academy of Science and Technology
1225:Journal of the American Chemical Society
1181:Journal of the American Chemical Society
1137:Journal of the American Chemical Society
1090:
875:Journal of the American Chemical Society
828:
744:Journal of the American Chemical Society
701:Journal of the American Chemical Society
658:Journal of the American Chemical Society
503:Korean Academy of Science and Technology
448:Korean Academy of Science and Technology
314:Copper-catalyzed multicomponent coupling
244:Journal of the American Chemical Society
225:(KAIST). He is also the director of the
1093:Angewandte Chemie International Edition
963:Angewandte Chemie International Edition
918:Angewandte Chemie International Edition
831:Angewandte Chemie International Edition
1661:
304:
294:as an associate editor of the journal
559:""학문의 대 잇는다"…KAIST '초세대 협업연구실' 추가 개소"
360:Sukbok Chang's gamma lactam synthesis
527:Fields-Hall, Mia (5 November 2019).
411:2017: 1st ACS-KCS Excellence Award,
402:2018: JSPS Invitational Fellowship,
364:
1392:
610:
583:
556:
13:
355:
317:
14:
1725:
1457:(in Korean). HelloDD. 2 July 2019
427:Alexander von Humboldt Foundation
1050:The Journal of Organic Chemistry
788:The Journal of Organic Chemistry
440:2015: Knowledge Creation Award,
334:
238:The Journal of Organic Chemistry
16:South Korean chemist (born 1962)
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370:2023: The Asian Scientist 100,
1449:"'최고과기인상'에 김기남 삼성전자·장석복 KAIST"
1395:"32회 삼성호암상…오용근 포스텍 교수 등 6인 수상"
735:
692:
645:
639:"Sukbok Chang's group website"
631:
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281:. He subsequently worked with
217:
158:
142:
1:
1709:South Korean organic chemists
924:(39): 9709–9721. 2012-09-19.
484:
269:in 1985, and M.S degree from
250:Accounts of Chemical Research
1563:(in Korean). 18 October 2018
29:
7:
1704:Institute for Basic Science
1615:Institute for Basic Science
1588:Institute for Basic Science
586:"KAIST, 초세대 협업연구실 2곳 추가 개소"
227:Institute for Basic Science
195:
181:
116:Institute for Basic Science
10:
1730:
255:C-H bond functionalization
1684:Harvard University alumni
1508:American Chemical Society
1367:"The Asian Scientist 100"
1337:10.1038/s41929-019-0230-x
537:American Chemical Society
413:American Chemical Society
390:
273:in 1987. Then, he joined
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1643:(in Korean). 4 July 2019
1637:"한림원 사람들/회원: 회원동정 (장석복)"
1022:10.15227/orgsyn.091.0052
1699:Korea University alumni
1694:Academic staff of KAIST
1535:Department of Chemistry
1481:Department of Chemistry
1293:10.1126/science.aap7503
611:한성형 (11 January 2023).
584:여용준 (11 January 2023).
557:노현섭 (11 January 2023).
423:Humboldt Research Award
417:Korean Chemical Society
1483:. KAIST. 27 April 2017
1105:10.1002/anie.201310544
975:10.1002/anie.201302784
930:10.1002/anie.201290068
843:10.1002/anie.200705940
380:Ho-Am Prize in Science
361:
349:
322:
291:Ewha Womans University
108:Ewha Womans University
359:
348:
321:
1237:10.1021/jacs.6b08211
1193:10.1021/jacs.5b01324
446:2014: Member of the
176:Revised Romanization
1393:이인준 (31 May 2022).
1284:2018Sci...359.1016H
1278:(6379): 1016–1021.
1231:(42): 14020–14029.
1056:(21): 11102–11109.
750:(46): 16046–16047.
617:Korea Lecturer News
454:Korea Science Award
436:Clarivate Analytics
305:Major contributions
86:Korea Science Award
1617:. 20 November 2019
1557:"장석복 KAIST 화학과 교수"
362:
350:
323:
279:Harvard University
72:Harvard University
1591:. 4 December 2018
1187:(13): 4534–4542.
1149:10.1021/ja501014b
1143:(11): 4141–4144.
1062:10.1021/jo4019683
1009:Organic Syntheses
969:(31): 8031–8036.
887:10.1021/ja303527m
881:(22): 9110–9113.
837:(15): 2836–2839.
800:10.1021/jo800733p
794:(14): 5520–5528.
756:10.1021/ja056399e
713:10.1021/ja0432968
670:10.1021/ja8026295
664:(29): 9254–9256.
365:Honors and awards
206:
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190:McCune–Reischauer
94:Scientific career
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283:Robert H. Grubbs
275:Eric N. Jacobsen
267:Korea University
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64:Korea University
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499:"회원: 장석복 (張碩福)"
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460:Kyung-Ahm Prize
373:Asian Scientist
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60:Alma mater
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1429:. 4 July 2019
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